天然气水合物含油气系统研究现状与展望`

doi:10.3969/j.issn.1006-6535.2021.01.001

特种油气藏 ›› 2021, Vol. 28 ›› Issue (1): 1-9.DOI: 10.3969/j.issn.1006-6535.2021.01.001

• 综述 • 下一篇

天然气水合物含油气系统研究现状与展望`

谭富荣^1,2,3, 耿庆明³, 刘世明³, 杜芳鹏⁴, 刘志武⁵

1.广东省新能源和可再生能源研究开发与应用重点实验室,广东广州 510640;
2.陕西省矿产地质调查中心,陕西西安 710068;
3.中国煤炭地质局,北京 100038;
4.西安科技大学,陕西西安 710054;
5.长安大学,陕西西安 710054

收稿日期:2019-10-10 修回日期:2020-11-02 出版日期:2021-02-25 发布日期:2021-04-27
通讯作者: 刘志武(1973—)男,副教授,1997年毕业于西安地质学院地质矿产勘查专业,2007年毕业于西北大学矿产普查与勘探专业,获博士学位,现从事沉积学与油气地质教学与科研工作。
作者简介:谭富荣(1984—),男,高级工程师,2008年毕业于河北工程大学资源勘查工程专业,2011年毕业于西北大学矿产普查与勘探专业,获硕士学位,现从事沉积盆地分析、油气地质研究工作。
基金资助:
国家自然科学基金“祁连山冻土区天然气水合物气源研究”(41702144);广东省新能源和可再生能源研究开发与应用重点实验室开放基金“祁连山冻土区天然气水合物气源研究——来自有机地球化学的证据”(Y807S91001);青海省地质调查局科研项目“柴北缘页岩气、铀等能源矿产潜力评价与靶区优选”( 2017042007ky007)

Research Status and Prospect of Natural Gas Hydrate Petroleum System

Tan Furong^1,2,3, Geng Qingming³, Liu Shiming³, Du Fangpeng⁴, Liu Zhiwu⁵

1. Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development, Guangzhou,Guangdong 510640,China;
2. Shaanxi Mineral Resources and Geological Survey,Xi'an,Shaanxi 710068,China;
3. China National Administration of Coal Geology,Beijing 100038,China;
4. Xi'an University of Science and Technology,Xi'an,Shaanxi 710054,China;
5. Chang'an University,Xi'an,Shaanxi 710054,China

Received:2019-10-10 Revised:2020-11-02 Online:2021-02-25 Published:2021-04-27

摘要/Abstract

摘要： 运用天然气水合物含油气系统理论,对天然气形成、分解这一复杂动态物理化学过程的研究进展进行了论述,分析了天然气水合物含油气系统的研究进展、存在问题和发展趋势,得到以下结论:大多数天然气水合物气源与生物降解密切相关;影响天然气水合物温度-压力临界曲线的主要因素为天然气、孔隙水的组分,地温梯度和冻土厚度不改变天然气水合物温度-压力临界曲线;天然气水合物含油气系统关键时刻的静态要素和动态过程以及两者之间的耦合关系在天然气水合物含油气系统中起重要作用。天然气水合物含油气系统研究不仅为天然气水合物成藏过程提供了理论依据,也为天然气水合物的勘探开发提供技术支持。

关键词: 天然气水合物, 含油气系统, 温度-压力临界曲线, 生物降解

Abstract: The theory of the natural gas hydrate petroleum system is applied to discusses the progress of research on the complex dynamic physicochemical process of natural gas formation and decomposition,the research progress,problems and development trend of the natural gas hydrate petroleum system are analyzed,and the following conclusions are obtained:most natural gas hydrate gas sources are closely related to the biodegradation; the main factors affecting the temperature-pressure critical curve of the natural gas hydrate are the components of natural gas and pore water,while the ground temperature gradient and permafrost thickness do not change the gas hydrate temperature-pressure critical curve; the static elements and dynamic processes at critical moments of the gas hydrate petroleum system and the coupling relationship between them play an important role in the gas hydrate petroleum system.The study of the gas hydrate petroleum system not only provides a theoretical basis for the process of gas hydrate accumulation,but also provides technical support for the exploration and development of gas hydrate.

Key words: natural gas hydrate, petroleum system, temperature-pressure critical curve, biodegradation

中图分类号:

谭富荣, 耿庆明, 刘世明, 杜芳鹏, 刘志武. 天然气水合物含油气系统研究现状与展望`[J]. 特种油气藏, 2021, 28(1): 1-9.

Tan Furong, Geng Qingming, Liu Shiming, Du Fangpeng, Liu Zhiwu. Research Status and Prospect of Natural Gas Hydrate Petroleum System[J]. Special Oil & Gas Reservoirs, 2021, 28(1): 1-9.

参考文献

[1] KVENVOLDEN K A.Gas hydrate geological perspective and global change[J].Reviews of Geophysics,1993,31(2):173-187.
[2] SLOAN E D.Clathrate hydrate of natural gases[M].2nd ed.New York:Marcel Dekker Inc.,1998:45-74.
[3] MAKOGON Y F,HOLDITCH S A,MAKOGON T Y.Natural gas hydrates:a potential energy source for the 21st Century[J].Journal of Petroleum Science & Engineering,2007,56(10):14-31.
[4] MAKOGON Y F.Natural gas hydrates:a promising source of energy[J].Journal of Natural Gas Science and Engineering,2010,2(1):49-59.
[5] BOSWELL R,ROSE K,COLLETT T S,et al.Geologic controls on gas hydrate occurrence in the Mount Elbert Prospect,Alaska North Slope[J].Marine and Petroleum Geology,2011,28(2):598-607.
[6] MILKOV A V.Economic geology of offshore gas hydrate accumulations and provinces[J].Marine and Petroleum Geology,2002,19(1):1-11.
[7] 吴时国,王秀娟,陈瑞新,等.天然气水合物地质概论[M].北京:科学出版社,2015:47-63
WU Shiguo,WANG Xiujuan,CHEN Ruixin,et al.An introduction to gas hydrate geology[M].Beijing:Science Press,2015:47-63.
[8] 吴能友,杨胜雄,王宏斌,等.南海北部陆坡神狐海域天然气水合物成藏的流体运移体系[J].地球物理学报,2009,52(6):1641-1650.
WU Nengyou,YANG Shengxiong,WANG Hongbin,et al.Gas-bearing fluid influx sub-system for gas hydrate geological system in Shenhu Area,northern south China Sea[J].Chinese Journal of Geophysics,2009,52(6):1641-1650.
[9] VADAKKEPULIYAMBATTA S,HORNBACH M J,BüNZ,S,et al.Controls on gas hydrate system evolution in a region of active fluid flow in the SW Barents Sea[J].Marine and Petroleum Geology,2015,66(4):861-872.
[10] 樊栓狮,关进安,梁德青,等.天然气水合物动态成藏理论[J].天然气地球科学,2007,18(6):819-826.
FAN Shuanshi,GUAN Jinan,LIANG Deqing,et al.A dynamic theory on natural gas hydrate reservoir formation[J].Natural Gas Geoscience,2007,18(6):819-826.
[11] 卢振权,吴能友,陈建文,等.试论天然气水合物成藏系统[J].现代地质,2008,22(3):363-375.
LU Zhenquan,WU Nengyou,CHEN Jianwen,et al.Preliminary discussion on gas hydrate Geological System[J].Geoscience,2008,22 (3):363-375.
[12] 翟刚毅,卢振权,卢海龙,等.祁连山冻土区天然气水合物成矿系统[J].矿物岩石,2014,34(4):79-92.
ZHAI Gangyi,LU Zhenquan,LU Hailong,et al.Gas hydrate geological system in the Qilian mountain permafrost[J].Journal of Mineral Petrology,2014,34(4):79-92.
[13] COOK A E,GOLDBERG D,KLEINBERG R L.Fracture-controlled gas hydrate systems in the northern Gulf of Mexico[J].Marine and Petroleum Geology,2008,25 (9):932-941.
[14] COLLETT T S,JOHNSON A,KNAPP C,et al.Natural gas hydrates:energy resource potential and associated geologic hazards[M].Memoir:American Association of Petroleum Geologists,2009:15-74.
[15] XU W,RUPPEL C.Predicting the occurrence,distribution,and evolution of methane gas hydrate in porous marine sediments[J].Journal of Geophysical Research Solid Earth,1999,104(B3):5081-5095.
[16] BHATNAGAR G,CHAPMAN W G,DICKENS G R,et al.Sulfate-methane transition as a proxy for average methane hydrate saturation in marine sediments[J].Geophysical Research Letters,2008,35(3):154-175.
[17] 张水昌,赵文智,李先奇,等.生物气研究新进展与勘探策略[J].石油勘探与开发,2005,32(4):90-96.
ZHANG Shuichang,ZHAO Wenzhi,LI Xianqi,et al.Advances in biogenic gas studies and play strategies[J].Petroleum Exploration and Development,2005,32(4):90-96.
[18] 吴后波,苏晓波,颜文.海底天然气水合物的微生物成因及识别[J].海洋科学,2008,32(3):96-100.
WU Houbo,SU Xiaobo,YAN Wen.The microbial genesis of submarine gas hydrate and its microbiological indication[J].Marine Sciences,2008,32(3):96-100.
[19] 辛碧霄,陈一俊.生物气成因机制与勘探前景[J].当代化工,2018,47(9):1928-1931.
XIN Bixiao,CHEN Yijun.Formation mechanism and exploration potential of biogenic gases[J].Contemporary Chemical Industry,2018,47(9):1928-1931.
[20] NOZHEVNIKOVA A N,HOLLIGER C,AMMANN A,et al.Met-
hanogenesis in sediments from deep lakes at different temperatures (2-70°C)[J].Water Science & Technology,1997,36(6/7):57-64.
[21] 李本亮,王明明,冉启贵,等.地层水含盐度对生物气运聚成藏的作用[J].天然气工业,2003,23(5):16-20.
LI Benliang,WANG Mingming,RAN Qigui,et al.Effect of the salinity of formation water on biogas migration,accumulation and reservoir formation[J].Natural Gas Industry,2003,23(5):16-20.
[22] 林春明,钱奕中.浙江沿海平原全新统气源岩特征及生物气形成的控制因素[J].沉积学报,1997,15(增刊):70-75.
LIN Chunming,QIAN Yizhong.Gas source rock features and controlling factors for biogas formation in Holocene series in Zhejiang Coastal Plain[J].Acta Sedimentologica Sinica,1997,15(S):70-75.
[23] 关德师.控制生物气富集成藏的基本地质因素[J].天然气工业,1997,17(5):8-12.
GUAN Deshi.Fundamental geologic factors controlling biogas accumulation[J].Natural Gas Industry,1997,17(5):8-12.
[24] 关德师,戚厚发,钱贻伯,等.生物气的生成演化模式[J].石油学报,1997,18(3):31-36.
GUAN Deshi,QI Houfa,Qian Yibo,et al.Generation and evolution model of biogenic gas[J].Acta Petroleum Sinica,1997,18(3):31-36.
[25] 刘若冰.浅层生物气特征、成藏条件与富集规律研究——以云南省曲靖盆地为例[D].成都:成都理工大学,2007.
LIU Ruobing.Study of the characteristics,reservoir conditions and enriched rules of shallow biogenic gases:take Qujing Basin as an example in Yunnan Province[D].Chengdu:Chengdu University of Technology,2007.
[26] 王新,裘俊红.笼形水合物研究与应用[J].化工生产与技术,2004,11(3):19-23.
WANG Xin,QIU Junhong.Research and application of cage hydrocarbons[J].Chemical Production and Technology,2004,11(3):19-23.
[27] 张俊霞,任建业.天然气水合物研究中的几个重要问题[J].地质科技情报,2001,20 (1):44-48.
ZHANG Junxia,REN Jianye.Several important problems in the research of gas hydrates[J].Geological Science and Technology Information,2001:20(1):44-48.
[28] RICZ D D.Relation of natural gas composition to thermal maturity and source rock type in San,Juan Basin,northwestern New Mexico and southwestern Colorado[J].AAPG Bulletin,1983,67(8):1199-1218.
[29] 周翥虹,周瑞年,管志强.柴达木盆地东部第四系气源岩地化特征与生物气前景 [J]. 石油勘探与开发,1994,21(2):30-36.
ZHOU Zhuhong,ZHOU Ruinian,GUAN Zhiqiang.Geochemical properties of source materials and biogas prospects of the Quaternary gas in east of Qaidam Basin[J].Petroleum exploration and development,1994,21(2):30-36.
[30] NOBLE R A,HENK F H.Hydrocarbon charge of a bacterial gas field by prolonged methanogenesis:an example from the last,Java Sea Indonesia[J].Organic Geochemistry,1998,29(1/2/3):301-314.
[31] KATZ B J,NARIMANOV A,HUSEINZADEH R.Significance of microbial processes in gases of the south Caspian Basin[J].Marine and Petroleum Geology,2002,19(6):783-796.
[32] 金庆焕,张光学,杨木壮.天然气水合物资源概论[M].北京:科学出版社,2006:45-67.
JIN Qinghuan,ZHANG Guanxue,YANG Muzhuang.General introduction to natural gas hydrate resources[M].Beijing:Science Press,2006:45-67.
[33] KHAN M N,WARRIER P,PETERS C J,et al.Advancements in hydrate phase equilibria and modeling of gas hydrates systems[J].Fluid Phase Equilibria,2018,463(1):48-61.
[34] KHAN M N,WARRIER P,PETERS C J,et al.Review of vapor-liquid equilibria of gas hydrate formers and phase equilibria of hydrates[J].Journal of Natural Gas Science and Engineering,2016,35(7):1388-1404.
[35] HOLDER G D,MALONE R D,LAWSON W F.Effects of gas composition and geothermal properties on the thickness and depth of natural-gas-hydrate zone [J].Journal of Petroleum Technology,1987,39(9):1147-1152.
[36] DICKENS G R,QUINBY-HUNT M S.Methane hydrate stability in seawater [J].Geophysical Research Letters,1994,21(19):2115-2118.
[37] 谭富荣,万余庆,吕俊娥,等.木里煤田聚乎更矿区侏罗系天然气水合物成藏要素分析[J].中国煤炭地质,2017,29(6):32-39.
TAN Furong,WAN Yuqing,LYU June,et al.Jurassic gas hydrate reservoir factors analysis in Juhugeng Mining Area,Muri Coalfield[J].Coal Geology of China,2017,29(6):32-39.
[38] HYNDMAN R D,DAVIS E E.A mechanism for the formation of methane hydrate and seafloor bottom-simulating reflectors by vertical fluid expulsion[J].Journal of Geophysical Research Solid Earth,1992,97(B5):7025-7041.
[39] COOK A E,GOLDBERG D.Extent of gas hydrate filled fracture planes:implications for in situ methanogenesis and resource potential[J].Geophysical Research Letters,2008,35(15):L15302.
[40] TORRES M E,WALLMANN K,TRéHU A M,et al.Gas hydrate growth,methane transport,and chloride enrichment at the southern summit of hydrate ridge,Cascadia margin off Oregon[J].Earth and Planetary Science Letters,2004,226(1/2):225 -241.
[41] TORRES M E,TRéHU A M,CESPEDES N,et al.Methane hydrate formation in turbidite sediments of northern Cascadia,ODP expedition 311[J].Earth and Planetary Science Letters,2008,271(1):170-180.
[42] 张鹏,吴青柏,蒋观利,等.不同颗粒介质内甲烷水合物形成反应特征 [J].天然气地球科学,2013,24(2):265-272.
ZHANG Peng,WU Qingbai,JIANG Guanli,et al.Formation reaction characteristics of methane hydrate in different granular media[J].Natural Gas Geoscience,2013,24(2):265-272.
[43] 苏明,乔少华,魏伟,等.墨西哥湾天然气水合物油气系统[J].新能源进展,2013,1(2):179-186.
SU Ming,QIAO Shaohua,WEI Wei,et al.The natural gas hydrate petroleum system in the Gulf of Mexico[J].Advances In New and Renewable Energy,2013,1(2):179-186.
[44] 肖红平,林畅松,彭涌,等.天然气水合物油气系统概念内涵及实例分析[J].地球科学进展,2017,32(1):21-33.
XIAO Hongping,LIN Changsong,PENG Yong,et al.Concept and intension of natural gas hydrate petroleum system and case analysis[J].Advances in Earth Science,2017,32(1):21-33.
[45] 丛晓荣,张伟,刘丽华,等.天然气水合物油气系统模拟新技术方法与应用[J].海洋地质前沿,2018,34(7):33-45.
CONG Xiaorong,ZHANG Wei,LIU Lihua,et al.New technology for gas hydrate petroleum system modeling and its application[J].Marine Geology Frontiers,2018,34(7):33-45.

天然气水合物含油气系统研究现状与展望`

Research Status and Prospect of Natural Gas Hydrate Petroleum System

PDF (PC)

可视化

摘要/Abstract

引用本文

使用本文

参考文献

相关文章 15

编辑推荐

Metrics

本文评价

[1]	孟大江, 路允乾, 张宝金, 王利杰. 叠前反演技术在天然气水合物储层预测中的应用[J]. 特种油气藏, 2023, 30(2): 51-57.
[2]	翟诚, 孙可明. 天然气水合物降压分解诱发储层变形破坏正交数值模拟实验研究[J]. 特种油气藏, 2022, 29(1): 99-106.
[3]	孙可明，王婷婷，翟诚，辛利伟，范楠. 不同饱和度天然气水合物加热分解界面变化规律[J]. 特种油气藏, 2018, 25(5): 129-.
[4]	付茜，刘世丽. 苏北盆地生物降解气特征及成藏模式[J]. 特种油气藏, 2018, 25(4): 57-.
[5]	孙林，杨万有，李旭光，杨淼. 天然气水合物酸化-自生热气开采技术研究[J]. 特种油气藏, 2018, 25(3): 149-.
[6]	孙可明，王婷婷，翟诚，罗慧玉. 天然气水合物加热分解储层变形破坏规律研究[J]. 特种油气藏, 2017, 24(5): 91-.
[7]	陈学海，卢双舫，陈学洋，薛海涛. 北乌斯丘尔特盆地含油气系统及勘探前景分析[J]. 特种油气藏, 2017, 24(3): 31-.
[8]	李一腾，叶加仁，曹强，刘一茗，刘中戎. 西藏伦坡拉盆地原油地球化学特征[J]. 特种油气藏, 2016, 23(3): 71-.
[9]	邓磊，文志刚，刘蕴，董纹希. 漠河盆地漠河组天然气水合物潜在气源岩评价[J]. 特种油气藏, 2015, 22(5): 31-.
[10]	蔡国刚鞠俊成. 辽河西部凹陷稠油成藏机制及深化勘探方法探讨[J]. , 2010, 17(4): 1-.
[11]	李芳芳刘晓栋. 天然气水合物开采新技术及其工业化开采的制约因素[J]. , 2010, 17(3): 1-.
[12]	白振华. 准噶尔盆地乌夏地区稠油稠变过程及成藏特征[J]. , 2009, 16(1): 1-.
[13]	霍进　吴运强　赵增义　李爱军　丁湘华. 准噶尔盆地风城地区稠油特征及其成因探讨[J]. , 2008, 15(2): 1-.
[14]	韩霞吴拓徐冠军李培新马玉东. 生物降解稠油油源对比新方法及其应用[J]. , 2007, 14(5): 1-.
[15]	邓柯　申艳　王宇. 天然气水合物预测模型研究的进展[J]. , 2006, 13(4): 1-.